Momentum Distributions from Strong-Field Ionization with Angular Streaking

Reconstructed 3D photoelectron momentum distribution, along with a sketch of the polarization ellipse and the beam route. (Tailored from Willenberg et al., Nat. Commun. 10, 5548; 2019). Credit score: ETH Zurich, D-PHYS, Keller group

The primary sub-femtosecond examine of the linear photon momentum switch throughout an ionization course of offers unprecedented perception into the beginning of photoelectrons.

The interplay between gentle and matter is the foundation of each many basic phenomena and numerous sensible applied sciences. Most famously, in the photoelectric impact, electrons are emitted from a cloth that’s uncovered to gentle of appropriate power. For lengthy, the origin of the phenomenon remained a riddle, and solely with the creation of quantum concept — and due to the genius of Albert Einstein — was the impact absolutely understood. Einstein acquired the 1921 Nobel Prize in Physics for his discovery of the underlying legal guidelines, and since then the impact has been harnessed in functions starting from spectroscopy to night-vision units. In some vital instances, the key precept is the switch not of power however of linear momentum — or, impulse — from photons to electrons. That is the case, as an example, when laser gentle is used to chill microscopic and macroscopic objects, or to grasp the phenomenon of radiation stress.

Regardless of the basic significance of momentum switch, the exact particulars of how gentle passes its impulse on to matter are nonetheless not absolutely understood. One cause is that the transferred impulse modifications throughout an optical cycle on extraordinarily quick, sub-femtosecond timescales. To this point, research revealed primarily data on time-averaged conduct, lacking time-dependent facets of the linear-momentum switch throughout photoionization. This hole has now been stuffed by the group of Ursula Keller at the Institute for Quantum Electronics, as they report in a paper printed right now (December 5, 2019) in Nature Communications.

Reconstructed 3D Photoelectron Momentum Distribution

Reconstructed 3D photoelectron momentum distribution, along with a sketch of the polarization ellipse and the beam route. (From Willenberg et al., Nat. Commun. 10, 5548; 2019). Credit score: ETH Zurich, D-PHYS, Keller group

They checked out the case of excessive laser intensities, the place a number of photons are concerned in the ionization course of, and investigated how a lot momentum is transferred in the route of laser propagation. To attain enough time decision, they employed the so-called attoclock method, which has been developed and refined in the Keller lab over the previous decade. On this methodology, attosecond time decision is achieved with out having to provide attosecond laser pulses. As an alternative, details about the rotating laser-field vector in near round polarised gentle is used to measure time relative to the ionization occasion with attosecond precision. Similar to the hand of a clock — simply now this clock hand is rotating by a full circle inside one optical cycle of 11.3-fs period.

With this versatile software at hand, the ETH physicists had been in a position to decide how a lot linear momentum electrons gained relying on when the photoelectrons had been ‘born.’ They discovered that the quantity of momentum transferred in the propagation route of the laser does certainly rely on when throughout the oscillation cycle of the laser the electron is ‘freed’ from the matter, of their case xenon atoms. Because of this at the very least for the situation they explored, the time-averaged radiation stress image shouldn’t be relevant. Intriguingly, they’ll reproduce the noticed conduct nearly absolutely inside a classical mannequin, whereas many eventualities of light-matter interplay, similar to Compton scattering, can solely be defined inside a quantum mechanical mannequin.

The classical mannequin needed to be prolonged although, to take note of the interplay between the outgoing photoelectron and the residual xenon ion. This interplay, they present of their experiments, induces an extra attosecond delay in the timing of the linear momentum switch in comparison with the theoretical prediction for a free electron born throughout the pulse. Whether or not such delays are a common property of photoionization or in the event that they apply just for the type of eventualities investigated in the current examine stays open for now. What is obvious, nonetheless, is that with this primary examine of linear momentum switch throughout ionization on the pure timescale of the course of, the Keller group opened up a brand new thrilling path to discover the very basic nature of light-matter interactions — thus making good on a central promise of attosecond science.

Reference: “Sub-cycle time resolution of multi-photon momentum transfer in strong-field ionization” by Benjamin Willenberg, Jochen Maurer, Benedikt W. Mayer and Ursula Keller, 5 December 2019, Nature Communications.
DOI: 10.1038/s41467-019-13409-6



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